They had a £22 million offer for the Tottenham playmaker turned down earlier this month, but had been hopeful he would move.
Having failed to convince the player, who is under contract, to leave his club, they have now made a huge offer for Palermo’s Argentine star.
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The reputation of the Premier League means it is the most popular and one of the most watched leagues in the world.
Five English clubs will compete in the last sixteen of the Champions League for the first time ever as Liverpool, Manchester United, Manchester City, Chelsea and Tottenham face some difficult away matches.