The Mexico forward, who used to play for Barcelona, is the club’s biggest signing of the summer so far.
“I am delighted to take this next step in my career, and finally to be able to play for Villarreal, a great club I was about to join last year before they were regrettably relegated,” Dos Santos told Villarreal’s website (www.villarrealcf.es).
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The reputation of the Premier League means it is the most popular and one of the most watched leagues in the world.
Five English clubs will compete in the last sixteen of the Champions League for the first time ever as Liverpool, Manchester United, Manchester City, Chelsea and Tottenham face some difficult away matches.